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Doubly indexed variables are often useful.
No easy construct exists like for simply indexed ones though.
That said, list comprehension makes it relatively easy.
Here is one way to obtain the requested indexing.
sage: α = [var(f"α_{i}_{j}", latex_name=fr"\alpha_{{{i},{j}}}")
....:      for i in range(3) for j in range(3)]
 Copyright Sage, 2010. Some rights reserved under creative commons license. Content on this site is licensed under a Creative Commons Attribution Share Alike 3.0 license.
 
                
                Copyright Sage, 2010. Some rights reserved under creative commons license. Content on this site is licensed under a Creative Commons Attribution Share Alike 3.0 license.